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Macrolorblx uniquely combines , room‑temperature self‑assembly , and ultrafast, reversible optical tuning , surpassing current bottom‑up PhC platforms.

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Author(s): A. R. Khan, J. L. Mendoza, H. S. Lee, K. T. O’Neil Affiliations: Department of Materials Science & Engineering, Institute for Advanced Photonics, Global University, 123 Innovation Way, City, Country Correspondence: a.khan@globaluniv.edu

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Samples were irradiated with (10 mW cm⁻²) for 60 s to induce trans→cis isomerization, then with 450 nm blue light to revert to trans. In‑situ reflectance tracked a blue‑shift of the stop‑band from 670 nm to 795 nm, confirming reversible tuning.

Recent work on has shown that molecular design can embed functional photonic motifs directly into the crystal lattice, enabling in situ tunability [6,7]. Inspired by these developments, we designed a macrocyclic platform that simultaneously offers (i) a rigid backbone for structural fidelity, (ii) photo‑responsive side‑chains for dynamic refractive‑index modulation, and (iii) high‑Z inorganic nodes for enhanced contrast. The resulting macrolorblx (MLX) molecules constitute a new class of self‑assembling photonic metamaterials .